Knowledge of aerosol size and composition is important for determining radiative forcing effects of aerosols, identifying aerosol sources and improving aerosol satellite retrieval algorithms. The ability to extrapolate aerosol size and composition, or type, from intensive aerosol optical properties can help expand the current knowledge of spatiotemporal variability in aerosol type globally, particularly where chemical composition measurements do not exist concurrently with optical property measurements. This study uses medians of the scattering (A) over circle ngstrom exponent (SAE), absorption (A) over circle ngstrom exponent (AAE) and single scattering albedo (SSA) from 24 stations within the NOAA/ESRL Federated Aerosol Monitoring Network to infer aerosol type using previously published aerosol classification schemes. Three methods are implemented to obtain a best estimate of dominant aerosol type at each station using aerosol optical properties. The first method plots station medians into an AAE vs. SAE plot space, so that a unique combination of intensive properties corresponds with an aerosol type. The second typing method expands on the first by introducing a multivariate cluster analysis, which aims to group stations with similar optical characteristics and thus similar dominant aerosol type. The third and final classification method pairs 3-day backward air mass trajectories with median aerosol optical properties to explore the relationship between trajectory origin (proxy for likely aerosol type) and aerosol intensive parameters, while allowing for multiple dominant aerosol types at each station. The three aerosol classification methods have some common, and thus robust, results. In general, estimating dominant aerosol type using optical properties is best suited for site locations with a stable and homogenous aerosol population, particularly continental polluted (carbonaceous aerosol), marine polluted (carbonaceous aerosol mixed with sea salt) and continental dust/biomass sites (dust and carbonaceous aerosol); however, current classification schemes perform poorly when predicting dominant aerosol type at remote marine and Arctic sites and at stations with more complex locations and topography where variable aerosol populations are not well represented by median optical properties. Although the aerosol classification methods presented here provide new ways to reduce ambiguity in typing schemes, there is more work needed to find aerosol typing methods that are useful for a larger range of geographic locations and aerosol populations.
Wells, K. C.; Millet, D. B.; Bousserez, N.; Henze, D. K.; Griffis, T. J.; Chaliyakunnel, S.; Dlugokencky, E. J.; Saikawa, E.; Xiang, G.; Prinn, R. G.; O'Doherty, S.; Young, D.; Weiss, R. F.; Dutton, G. S.; Elkins, J. W.; Krummel, P. B.; Langenfelds, R.; Steele, L. P.;
Published Date:
2018
Source:
Atmospheric Chemistry and Physics, 18(2), 735-756.
Description:
We present top-down constraints on global monthly N2O emissions for 2011 from a multi-inversion approach and an ensemble of surface observations. The inversions employ the GEOS-Chem adjoint and an array of aggregation strategies to test how well curr...
Raczka, B.; Biraud, S. C.; Ehleringer, J. R.; Lai, C. T.; Miller, J. B.; Pataki, D. E.; Saleska, S. R.; Torn, M. S.; Vaughn, B. H.; Wehr, R.; Bowling, D. R.;
Published Date:
2017
Source:
Journal of Geophysical Research-Biogeosciences, 122(8), 1969-1987.
Description:
The seasonal pattern of the carbon isotope content (delta C-13) of atmospheric CO2 depends on local and nonlocal land-atmosphere exchange and atmospheric transport. Previous studies suggested that the delta C-13 of the net land-atmosphere CO2 flux (d...
Journal of Geophysical Research-Atmospheres, 123(15), 7950-7973.
Description:
In this study, we analyze a set of agroclimatological indices across West Africa and assess their projected changes for the future. We apply the regional climate model CCLM (COnsortium for Small-scale MOdelling in CLimate Mode) with a high spatial re...
Kenagy, H. S.; Sparks, T. L.; Ebben, C. J.; Wooldrige, P. J.; Lopez-Hilfiker, F. D.; Lee, B. H.; Thornton, J. A.; McDuffie, E. E.; Fibiger, D. L.; Brown, S. S.; Montzka, D. D.; Weinheimer, A. J.; Schroder, J. C.; Campuzano-Jost, P.; Day, D. A.; Jimenez, J. L.; Dibb, J. E.; Campos, T.; Shah, V.; Jaegle, L.; Cohen, R. C.;
Published Date:
2018
Source:
Journal of Geophysical Research-Atmospheres, 123(17), 9813-9827.
Description:
Although urban NOx lifetimes have been examined extensively during summertime conditions, wintertime NOx chemistry has been comparatively less studied. We use measurements of NOx and its oxidation products from the aircraft-based WINTER (Wintertime I...
Jarvinen, E.; Ignatius, K.; Nichman, L.; Kristensen, T. B.; Fuchs, C.; Hoyle, C. R.; Hoppel, N.; Corbin, J. C.; Craven, J.; Duplissy, J.; Ehrhart, S.; El Haddad, I.; Frege, C.; Gordon, H.; Jokinen, T.; Kallinger, P.; Kirkby, J.; Kiselev, A.; Naumann, K. H.; Petaja, T.; Pinterich, T.; Prevot, A. S. H.; Saathoff, H.; Schiebel, T.; Sengupta, K.; Simon, M.; Slowik, J. G.; Trostl, J.; Virtanen, A.; Vochezer, P.; Vogt, S.; Wagner, A. C.; Wagner, R.; Williamson, C.; Winkler, P. M.; Yan, C.; Baltensperger, U.; Donahue, N. M.; Flagan, R. C.; Gallagher, M.; Hansel, A.; Kulmala, M.; Stratmann, F.; Worsnop, D. R.; Mohler, O.; Leisner, T.; Schnaiter, M.;
Published Date:
2016
Source:
Atmospheric Chemistry and Physics, 16(7), 4423-4438.
Description:
Under certain conditions, secondary organic aerosol (SOA) particles can exist in the atmosphere in an amorphous solid or semi-solid state. To determine their relevance to processes such as ice nucleation or chemistry occurring within particles requir...
Butler, R.; Palmer, P. I.; Feng, L.; Andrews, S. J.; Atlas, E. L.; Carpenter, L. J.; Donets, V.; Harris, N. R. P.; Montzka, S. A.; Pan, L. L.; Salawitch, R. J.; Schauffler, S. M.;
Published Date:
2018
Source:
Atmospheric Chemistry and Physics, 18(17), 13135-13153.
Description:
We use the GEOS-Chem global 3-D atmospheric chemistry transport model to interpret atmospheric observations of bromoform (CHBr3) and dibromomethane (CH2Br2) collected during the CAST and CONTRAST aircraft measurement campaigns over the western Pacifi...
Fried, A.; Barth, M. C.; Bela, M.; Weibring, P.; Richter, D.; Walega, J.; Li, Y.; Pickering, K.; Apel, E.; Hornbrook, R.; Hills, A.; Riemer, D. D.; Blake, N.; Blake, D. R.; Schroeder, J. R.; Luo, Z. J.; Crawford, J. H.; Olson, J.; Rutledge, S.; Betten, D.; Biggerstaff, M. I.; Diskin, G. S.; Sachse, G.; Campos, T.; Flocke, F.; Weinheimer, A.; Cantrell, C.; Pollack, I.; Peischl, J.; Froyd, K.; Wisthaler, A.; Mikoviny, T.; Woods, S.;
Published Date:
2016
Source:
Journal of Geophysical Research-Atmospheres, 121(12), 7430-7460.
Description:
We have developed semi-independent methods for determining CH2O scavenging efficiencies (SEs) during strong midlatitude convection over the western, south-central Great Plains, and southeastern regions of the United States during the 2012 Deep Convec...
Janssens-Maenhout, G.; Crippa, M.; Guizzardi, D.; Dentener, F.; Muntean, M.; Pouliot, G.; Keating, T.; Zhang, Q.; Kurokawa, J.; Wankmuller, R.; van der Gon, H. D.; Kuenen, J. J. P.; Klimont, Z.; Frost, G.; Darras, S.; Koffi, B.; Li, M.;
Published Date:
2015
Source:
Atmospheric Chemistry and Physics, 15(19), 11411-11432.
Description:
The mandate of the Task Force Hemispheric Transport of Air Pollution (TF HTAP) under the Convention on Long-Range Transboundary Air Pollution (CLRTAP) is to improve the scientific understanding of the intercontinental air pollution transport, to quan...
Brown, S. S.; Dube, W. P.; Tham, Y. J.; Zha, Q. Z.; Xue, L. K.; Poon, S.; Wang, Z.; Blake, D. R.; Tsui, W.; Parrish, D. D.; Wang, T.;
Published Date:
2016
Source:
Journal of Geophysical Research-Atmospheres, 121(5), 2457-2475.
Description:
Nighttime reactions of nitrogen oxides influence ozone, volatile organic compounds, and aerosol and are thus important to the understanding of regional air quality. Despite large emissions and rapid recent growth of nitrogen oxide concentrations, the...
Kim, J.; Johnson, L. E.; Cifelli, R.; Choi, J.; Chandrasekar, V.;
Published Date:
2018
Source:
Water, 10(7), 21.
Description:
Soil moisture retention (SMR) capacity plays a key role in estimating the direct runoff when a multi-pulse storm event occurs. It is very important to know how much SMR will be recovered during the intervals of no rain of a multi-pulse storm. This st...
Fairall, C. W.; Matrosov, S. Y.; Williams, C. R.; Walsh, E. J.;
Published Date:
2018
Source:
Journal of Atmospheric and Oceanic Technology, 35(3), 593-608.
Description:
The NOAA W-band radar was deployed on a P-3 aircraft during a study of storm fronts off the U.S. West Coast in 2015 in the second CalWater (CalWater-2) field program. This paper presents an analysis of measured equivalent radar reflectivity factor Z(...
A 4-year record of aerosol size and hygroscopic growth factor distributions measured at the Department of Energy's Southern Great Plains (SGP) site in Oklahoma, U.S. were used to estimate supersaturation (S)-dependent cloud condensation nuclei concen...
Mahoney, K.; Swales, D.; Mueller, M. J.; Alexander, M.; Hughes, M.; Malloy, K.;
Published Date:
2018
Source:
Journal of Climate, 31(16), 6281-6297.
Description:
Atmospheric rivers (ARs) are well-known producers of precipitation along the U.S. West Coast. Depending on their intensity, orientation, and location of landfall, some ARs penetrate inland and cause heavy rainfall and flooding hundreds of miles from ...
Dimdore-Miles, O. B.; Palmer, P. I.; Bruhwiler, L. P.;
Published Date:
2018
Source:
Atmospheric Chemistry and Physics, 18(24), 17895-17907.
Description:
We consider the utility of the annual inter-polar difference (IPD) as a metric for changes in Arctic emissions of methane (CH4). The IPD has been previously defined as the difference between weighted annual means of CH4 mole fraction data collected a...
Sea surface temperature anomalies (SSTA) in portions of the extratropics are known to recur from one winter to the next without persisting through the intervening summer. Previous studies identified only a limited number of midlatitude regions where ...
Richardson, K.; Asmutis-Silvia, R.; Drinkwin, J.; Gilardi, K. V. K.; Giskes, I.; Jones, G.; O'Brien, K.; Pragnell-Raasch, H.; Ludwig, L.; Antonelis, K.; Barco, S.; Henry, A.; Knowlton, A.; Landry, S.; Mattila, D.; MacDonald, K.; Moore, M.; Morgan, J.; Robbins, J.; van der Hoop, J.; Hogan, E.;
Published Date:
2019
Source:
Marine Pollution Bulletin, 138, 222-229.
Description:
Abandoned, lost or discarded fishing gear (ALDFG) comprises a significant amount of global marine debris, with diverse impacts to marine environments, wildlife, and the fishing industry. Building evidence on ALDFG is critical to holistically understa...
Smith, M.; Stammerjohn, S.; Persson, O.; Rainville, L.; Liu, G. Q.; Perrie, W.; Robertson, R.; Jackson, J.; Thomson, J.;
Published Date:
2018
Source:
Journal of Geophysical Research-Oceans, 123(5), 3164-3185.
Description:
High-resolution measurements of the air-ice-ocean system during an October 2015 event in the Beaufort Sea demonstrate how stored ocean heat can be released to temporarily reverse seasonal ice advance. Strong on-ice winds over a vast fetch caused mixi...
Chakraborty, A.; Ervens, B.; Gupta, T.; Tripathi, S. N.;
Published Date:
2016
Source:
Journal of Geophysical Research-Atmospheres, 121(8), 4317-4332.
Description:
Size-resolved fog water samples were collected in two consecutive winters at Kanpur, a heavily polluted urban area of India. Samples were analyzed by an aerosol mass spectrometer after drying and directly in other instruments. Residues of fine fog dr...
Kim, P. S.; Jacob, D. J.; Fisher, J. A.; Travis, K.; Yu, K.; Zhu, L.; Yantosca, R. M.; Sulprizio, M. P.; Jimenez, J. L.; Campuzano-Jost, P.; Froyd, K. D.; Liao, J.; Hair, J. W.; Fenn, M. A.; Butler, C. F.; Wagner, N. L.; Gordon, T. D.; Welti, A.; Wennberg, P. O.; Crounse, J. D.; St. Clair, J. M.; Teng, A. P.; Millet, D. B.; Schwarz, J. P.; Markovic, M. Z.; Perring, A. E.;
Heiblum, R. H.; Altaratz, O.; Koren, I.; Feingold, G.; Kostinski, A. B.; Khain, A. P.; Ovchinnikov, M.; Fredj, E.; Dagan, G.; Pinto, L.; Yaish, R.; Chen, Q.;
Published Date:
2016
Source:
Journal of Geophysical Research-Atmospheres, 121(11), 6336-6355.
Description:
We study the evolution of warm convective cloud fields using large eddy simulations of continental and trade cumulus. Individual clouds are tracked a posteriori from formation to dissipation using a 3-D cloud-tracking algorithm, and results are prese...
Japngie-Green, Crystal M.; Andrews, Elisabeth; McCubbin, Ian B.; Ogren, John A.; Hallar, Anna G.;
Published Date:
2019
Source:
Aerosol And Air Quality Research, 19(6), 1205-1213
Description:
Aerosols create large uncertainty in the planetary energy balance due to both direct and indirect radiative forcing. Understanding aerosol seasonal patterns is essential for accurate climate change prediction, but mountain regions are often difficult...
Park, Soojin; Kim, Sang-Woo; Lin, Neng-Huei; Pani, Shantanu Kumar; Sheridan, Patrick J.; Andrews, Elisabeth;
Published Date:
2019
Source:
Aerosol Air Qual. Res. 19: 1272-1283
Description:
We investigated the variability of in-situ and columnar aerosol optical properties (AOPs) at two regional background sites in the Asian continental outflow from 2012 to 2014. The monthly variability of the AOPs at each site is described in terms of i...