Details:

Journal Title:
Atmospheric Chemistry and Physics
Personal Author:
Manfred, Katherine M. ; Washenfelder, Rebecca A. ; Wagner, Nicholas L. ; Adler, Gabriela ; Erdesz, Frank ; ... More +
Manfred, Katherine M. ; Washenfelder, Rebecca A. ; Wagner, Nicholas L. ; Adler, Gabriela ; Erdesz, Frank ; Womack, Caroline C. ; Lamb, Kara D. ; Schwarz, Joshua P. ; Franchin, Alessandro ; Selimovic, Vanessa ; Yokelson, Robert J. ; Murphy, Daniel M. Less -
NOAA Program & Office:
OAR (Oceanic and Atmospheric Research) ; ESRL (Earth System Research Laboratory) ; CSL (Chemical Sciences Laboratory) ; CIRES (Cooperative Institute for Research in Environmental Sciences)
OAR (Oceanic and Atmospheric Research) ; ESRL (Earth System Research Laboratory) ; CSL (Chemical Sciences Laboratory) ; CIRES (Cooperative Institute for Research in Environmental Sciences) Less -
Description:
Particle morphology is an important parameter affecting aerosol optical properties that are relevant to climate and air quality, yet it is poorly constrained due to sparse in situ measurements. Biomass burning is a large source of aerosol that generates particles with different morphologies. Quantifying the optical contributions of non-spherical aerosol populations is critical for accurate radiative transfer models, and for correctly interpreting remote sensing data. We deployed a laser imaging nephelometer at the Missoula Fire Sciences Laboratory to sample biomass burning aerosol from controlled fires during the FIREX intensive laboratory study. The laser imaging nephelometer measures the unpolarized scattering phase function of an aerosol ensemble using diode lasers at 375 and 405 nm. Scattered light from the bulk aerosol in the instrument is imaged onto a charge- coupled device (CCD) using a wide-angle field-of-view lens, which allows for measurements at 4-175 degrees scattering angle with similar to 0.5 degrees angular resolution. Along with a suite of other instruments, the laser imaging nephelometer sampled fresh smoke emissions both directly and after removal of volatile components with a thermodenuder at 250 degrees C. The total integrated aerosol scattering signal agreed with both a cavity ring-down photoacoustic spectrometer system and a traditional integrating nephelometer within instrumental uncertainties. We compare the measured scattering phase functions at 405 nm to theoretical models for spherical (Mie) and fractal (Rayleigh-Debye-Gans) particle morphologies based on the size distribution reported by an optical particle counter. Results from representative fires demonstrate that particle morphology can vary dramatically for different fuel types. In some cases, the measured phase function cannot be described using Mie theory. This study demonstrates the capabilities of the laser imaging nephelometer instrument to provide realtime, in situ information about dominant particle morphology, which is vital for understanding remote sensing data and accurately describing the aerosol population in radiative transfer calculations.
Source:
Atmospheric Chemistry and Physics, 18(3), 1879-1894.
DOI:
https://doi.org/10.5194/acp-18-1879-2018
Document Type:
Journal Article
Rights Information:
CC BY
Compliance:
Submitted
Main Document Checksum:
[+]
urn:sha256:65f30015f157b2f3f085ca2ed64bd7f6ca8181f5c3b3b193ab25367edb64be95
Download URL:
https://repository.library.noaa.gov/view/noaa/21729/noaa_21729_DS1.pdf
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