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Assessing stratospheric transport in the CMAM30 simulations using ACE-FTS measurements
  • Published Date:
    2018
  • Source:
    Atmospheric Chemistry and Physics, 18(9), 6801-6828.
Filetype[PDF-4.42 MB]


Details:
  • Personal Author:
  • Description:
    Stratospheric transport in global circulation models and chemistry-climate models is an important component in simulating the recovery of the ozone layer as well as changes in the climate system. The Brewer-Dobson circulation is not well constrained by observations and further investigation is required to resolve uncertainties related to the mechanisms driving the circulation. This study has assessed the specified dynamics mode of the Canadian Middle Atmosphere Model (CMAM30) by comparing to the Atmospheric Chemistry Experiment Fourier transform spectrometer (ACE-FTS) profile measurements of CFC-11 (CCl3F), CFC-12 (CCl2F2), and N2O. In the CMAM30 specified dynamics simulation, the meteorological fields are nudged using the ERA-Interim reanalysis and a specified tracer was employed for each species, with hemispherically defined surface measurements used as the boundary condition. A comprehensive sampling technique along the line of sight of the ACE-FTS measurements has been utilized to allow for direct comparisons between the simulated and measured tracer concentrations. The model consistently overpredicts tracer concentrations of CFC-11, CFC-12, and N2O in the lower stratosphere, particularly in the northern hemispheric winter and spring seasons. The three mixing barriers investigated, including the polar vortex, the extratropical tropopause, and the tropical pipe, show that there are significant inconsistencies between the measurements and the simulations. In particular, the CMAM30 simulation underpredicts mixing efficiency in the tropical lower stratosphere during the June-July-August season.
  • DOI:
    http://dx.doi.org/10.5194/acp-18-6801-2018
  • Document Type:
    Journal Article
  • Collection(s):
    NOAA Cooperative Institutes
    Office of Oceanic and Atmospheric Research (OAR)
  • Main Document Checksum:
  • Supporting Files:
    No Additional Files
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      Source:
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      Description:
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      Description:
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      Description:
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      Description:
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      Description:
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      Source:
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      Description:
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      File Type:
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      Description:
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      2017
      Source:
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      Description:
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      Description:
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      Description:
      Organic nitrates in both gas and condensed (aerosol) phases were measured during the Uintah Basin Winter Ozone Study from January to February in 2012. A high degree of correlation between total aerosol volume at diameters less than 500 nm and the par...
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      Feingold, G.; Koren, I.; Yamaguchi, T.; Kazil, J.;
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      2015
      Source:
      Atmospheric Chemistry and Physics, 15(13), 7351-7367.
      Description:
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      2015
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      Atmospheric Chemistry and Physics, 15(19), 11411-11432.
      Description:
      The mandate of the Task Force Hemispheric Transport of Air Pollution (TF HTAP) under the Convention on Long-Range Transboundary Air Pollution (CLRTAP) is to improve the scientific understanding of the intercontinental air pollution transport, to quan...
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      Personal Author:
      Ervens, B.; Renard, P.; Tlili, S.; Ravier, S.; Clement, J. L.; Monod, A.;
      Published Date:
      2015
      Source:
      Atmospheric Chemistry and Physics, 15(16), 9109-9127.
      Description:
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      2015
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      Atmospheric Measurement Techniques, 8(3), 1575-1591.
      Description:
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