Details:

Journal Title:
Atmospheric Chemistry and Physics
Personal Author:
Brock, Charles A. ; Wagner, Nicholas L. ; Anderson, Bruce E. ; Beyersdorf, Andreas ; Campuzano-Jost, Pedro ; ... More +
Brock, Charles A. ; Wagner, Nicholas L. ; Anderson, Bruce E. ; Beyersdorf, Andreas ; Campuzano-Jost, Pedro ; Day, Douglas A. ; Diskin, Glenn S. ; Gordon, Timothy D. ; Jimenez, Jose L. ; Lack, Daniel A. ; Liao, Jin ; Markovic, Milos Z. ; Middlebrook, Ann M. ; Perring, Anne E. ; Richardson, Matthews S. ; Schwarz, Joshua P. ; Welti, Andre ; Ziemba, Luke D. ; Murphy, Daniel M. Less -
NOAA Program & Office:
OAR (Oceanic and Atmospheric Research) ; ESRL (Earth System Research Laboratory) ; CIRES (Cooperative Institute for Research in Environmental Sciences) ; CSL (Chemical Sciences Laboratory)
OAR (Oceanic and Atmospheric Research) ; ESRL (Earth System Research Laboratory) ; CIRES (Cooperative Institute for Research in Environmental Sciences) ; CSL (Chemical Sciences Laboratory) Less -
Description:
Aircraft observations of meteorological, trace gas, and aerosol properties were made between May and September 2013 in the southeastern United States (US). Regionally representative aggregate vertical profiles of median and interdecile ranges of the measured parameters were constructed from 37 individual aircraft profiles made in the afternoon when a well-mixed boundary layer with typical fair-weather cumulus was present (Wagner et al., 2015). We use these 0-4aEuro-km aggregate profiles and a simple model to calculate the sensitivity of aerosol optical depth (AOD) to changes in dry aerosol mass, relative humidity, mixed-layer height, the central diameter and width of the particle size distribution, hygroscopicity, and dry and wet refractive index, while holding the other parameters constant. The calculated sensitivity is a result of both the intrinsic sensitivity and the observed range of variation in these parameters. These observationally based sensitivity studies indicate that the relationship between AOD and dry aerosol mass in these conditions in the southeastern US can be highly variable and is especially sensitive to relative humidity (RH). For example, calculated AOD ranged from 0.137 to 0.305 as the RH was varied between the 10th and 90th percentile profiles with dry aerosol mass held constant. Calculated AOD was somewhat less sensitive to aerosol hygroscopicity, mean size, and geometric standard deviation, sigma(g). However, some chemistry-climate models prescribe values of sigma(g) substantially larger than we or others observe, leading to potential high biases in model-calculated AOD of aEuro-25aEuro-%. Finally, AOD was least sensitive to observed variations in dry and wet aerosol refractive index and to changes in the height of the well-mixed surface layer. We expect these findings to be applicable to other moderately polluted and background continental air masses in which an accumulation mode between 0.1-0.5aEuro-A mu m diameter dominates aerosol extinction.
Source:
Atmospheric Chemistry and Physics, 16(8), 5009-5019.
DOI:
https://doi.org/10.5194/acp-16-5009-2016
Document Type:
Journal Article
Rights Information:
CC BY
Compliance:
Submitted
Main Document Checksum:
[+]
urn:sha256:9ff25181c324a2ff383bb0071632c3fe29564a34931a5e8d223dc1e4e19d8a6d
Download URL:
https://repository.library.noaa.gov/view/noaa/22104/noaa_22104_DS1.pdf
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