Impact of high-resolution sea surface temperature, emission spikes and wind on simulated surface ozone in Houston, Texas during a high ozone episode
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2017
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Details
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Journal Title:Atmospheric Environment
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Description:Model-measurement comparisons for surface ozone often show significant error, which could be attributed to problems in meteorology and emissions fields. A WRF-SMOKE-CMAQ air quality modeling system was used to investigate the contributions of these inputs. In this space, a base WRF run (BASE) and a WRF run initializing with NOAA GOES satellite sea surface temperature (SST) (SENS) were performed to clarify the impact of high-resolution SST on simulated surface ozone (O3) over the Greater Houston area during 25 September 2013, corresponding to the high O3 episode during the NASA DISCOVER-AQ Texas campaign. The SENS case showed reduced land-sea thermal contrast during early morning hours due to 1–2 °C lower SST over water bodies. The lowered SST reduced the model wind speed and slowed the dilution rate. These changes led to a simulated downwind O3 change of ∼5 ppb near the area over land with peak simulated afternoon O3. However, the SENS case still under-predicted surface O3 in urban and industrial areas. Episodic flare emissions, dry sunny postfrontal stagnated conditions, and land-bay/sea breeze transitions could be the potential causes of the high O3.
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Content Notes:Authors acknowledge the free use of the NOAA GOES SST, NDBC buoy temperature and MADIS ACARS wind profiles data, NCEP NARR data, TCEQ CAMS in-situ meteorological and chemical species data, and NASA DISCOVER-AQ aircraft O3, NOy and HCHO data.
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Source:Atmospheric Environment, 152, 362-376
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DOI:
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ISSN:1352-2310
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Rights Information:Accepted Manuscript
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Rights Statement:The contents of the paper are the authors' sole responsibility. They do not represent the views of the TCEQ and NOAA or their staff.
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Compliance:Library
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Main Document Checksum:urn:sha256:c6361131fa5b61c7d18c7abbc4262bf3ba20af34042969b73054f4585898ed01
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