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Journal Title:Atmosphere
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Description:This work presents new climate and emissions scenarios to investigate changes on future meteorology and air quality in the U.S. Here, we employ a dynamically downscaled Weather Research and Forecasting model coupled with chemistry (WRF/Chem) simulations that use two Intergovernmental Panel on Climate Change scenarios (i.e., A1B and B2) integrated with explicitly projected emissions from a novel Technology Driver Model (TDM). The projected 2046–2055 emissions show widespread reductions in most gas and aerosol species under both TDM/A1B and TDM/B2 scenarios over the U.S. The WRF/Chem simulations show that under the combined effects of the TDM/A1B climate and emission changes, the maximum daily average 8-h ozone (MDA8 h O3) increases by ~3 ppb across the U.S. mainly due to widespread increases in near-surface temperature and background methane concentrations, with some contributions from localized TDM emission changes near urban centers. For the TDM/B2 climate and emission changes, however, the MDA8 h O3 is widely decreased, except near urban centers where the relative TDM emission changes and O3 formation regimes leads to increased O3. The number of O3 exceedance days (i.e., MDA8 h O3 > 70 ppb) for the entire domain is significantly reduced by a grid cell maximum of up to 43 days (domain average ~0.5 days) and 62 days (domain average ~2 days) for the TDM/A1B and TDM/B2 scenarios, respectively, while in the western U.S., larger O3 increases lead to increases in nonattainment areas, especially for the TDM/A1B scenario. The combined effects of climate and emissions (for both A1B and B2 scenarios) will lead to widespread decreases in the daily 24-h average (DA24 h) PM2.5 concentrations, especially in the eastern U.S. (max decrease up to 93 µg m−3). The PM2.5 changes are dominated by decreases in anthropogenic emissions for both the TDM/A1B and TDM/B2 scenarios, with secondary effects on decreasing PM2.5 from climate change. The number of PM2.5 exceedance days (i.e., DA24 h PM2.5 > 35 µg m−3) is significantly reduced over the eastern U.S. under both TDM/A1B and B2 scenarios, which suggests that both climate and emission changes may synergistically lead to decreases in PM2.5 nonattainment areas in the future.
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Source:Atmosphere 2023, 14(2), 225
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Rights Information:CC BY
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