Aerosols have a profound impact on cloud microphysics through their ability to serve as ice nucleating particles (INPs). As a result, cloud radiative properties and precipitation processes can be modulated by such aerosolcloud interactions. However, one of the largest uncertainties associated with atmospheric processes is the indirect effect of aerosols on clouds. The need for more advanced observations of INPs in the atmospheric vertical profile is apparent, yet most ice nucleation measurements are conducted on the ground or during infrequent and intensive airborne field campaigns. Here, we describe a novel measurement platform that is less expensive and smaller (< 5 kg) when compared to traditional aircraft and tethered balloon platforms and that can be used for evaluating two modes of ice nucleation (i.e., immersion and deposition). HOVERCAT (Honing On VERtical Cloud and Aerosol properTies) flew during a pilot study in Colorado, USA, up to 2.6 km above mean sea level (1.1 km above ground level) and consists of an aerosol module that includes an optical particle counter for size distributions (0.38-17 mu m in diameter) and a new sampler that collects up to 10 filter samples for offline ice nucleation and aerosol analyses on a launched balloon platform. During the May 2017 test flight, total particle concentrations were highest closest to the ground (up to 50 cm(-3) at < 50m above ground level) and up to 2 in 102 particles were ice nucleation active in the immersion mode (at 23 degrees C). The warmest temperature immersion and deposition mode INPs (observed up to -6 and -40.4 degrees C, respectively) were observed closest to the ground, but overall INP concentrations did not exhibit an inverse correlation with increasing altitude. HOVERCAT is a prototype that can be further modified for other airborne platforms, including tethered balloon and unmanned aircraft systems. The versatility of HOVERCAT affords future opportunities to profile the atmospheric column for more comprehensive evaluations of aerosol-cloud interactions. Based on our test flight experiences, we provide a set of recommendations for future deployments of similar measurement systems and platforms.

http://dx.doi.org/10.5194/amt-11-3969-2018

Journal Article